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John Michener's avatar

I have seen a lot of people worry about the radiation hazard of depleted Uranium to populations.

I could care less - Uranium is quite toxic as a chemical. The chemical hazard of Uranium to people is far far higher than its radiation hazard, enough so that any sane risk calculation would ignore the risk contribution from the radiation - the radiation portion of the risk is far smaller than the uncertainty in the associated chemical hazards.

I was a safety officer in a chemical process lab > 50 years ago. I remember a meeting where a very old bottle of a particularily dangerous chemical was found on a shelf. Nobody knew about it. One chemist was worried that it was a carcinogen. The old expert's comment was - 'who cares, that stuff is classified as a chemical weapon. It will kill you long before you get cancer from it."

In terms of risk to life, property and large scale destruction, I worry about dam failures.

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Jaro Franta's avatar

Similar sort of misinformation going on in Canada, no surprise.

It comes mostly from perennial antinuke activist Gordon Edwards, who frequently presents himself as Canadian Coalition for Nuclear Responsibility (CCNR).

He regularly receives "intervenor" funding from the CNSC - Canadian Nuclear Safety Commission - either directly or by contract from various antinuke groups, such as CELA (Canadian Environmental Law Association).

In recent years, Edwards has been campaigning against Canada’s project for used CANDU fuel disposal in a DGR (Deep Geological Repository), which is now slated to be built in western Ontario, about 30km west of the town of Ignace – which applied to participate in the site selection process 15 years ago, and voted overwhelmingly in favor of “hosting” the project early last year (2024).

Needless to say, Edwards’ scare mongering includes “the I-129 problem” – see linked picture below, which is a screen grab from a YouTube video from one of Edwards’ presentations last year.

Edwards also includes “the Cs-135 problem”.

https://cdn-images-1.medium.com/v2/resize:fit:1500/1*oG8Uka43J0Z_98ld_xYXqQ.png

My comments on Edwards’ claims were as follows:

First of all, it’s rare that nuclear fuel bundles have so much as a pinhole defect: When one does, it is immediately detected in the reactor, and the defective fuel bundle is removed.

Secondly, the thermal conditions inside the reactor are pretty fierce, with 300°C and high-pressure, high-velocity flow.

Once the defective fuel bundle is removed and placed into the cooling pool for storage, it stops leaking, because the thermal conditions are benign.

Used nuclear fuel bundles are barely warm, after 50 to 70 years of surface storage, whereas the boiling point of Iodine is 184.3°C, and for Cesium the boiling point is 671°C.

Perhaps more importantly, Edwards is talking about the extremely long-live isotope Iodine-129, not the short-lived isotope Iodine-131.

Iodine-131 is of concern in reactor operation, but NOT in long-term storage: It is completely gone in a few months following removal from the reactor. Iodine-129 remains in the used fuel for a very long time, but its radioactivity is extremely low: Canada’s nuclear regulator, the CNSC, requires prophylactic iodine pill distribution in the vicinity of nuclear power plants, but does NOT require their distribution around long-term used fuel storage sites, because the remaining Iodine-129 is insignificant, and there is no possibility of a million used fuel bundles getting pulverised while in storage – at least not until the next ice age, with the advancement of thick glaciers.

Third, let’s not forget – as Edwards does every time – that used CANDU fuel is 99% natural uranium, with just 0.6% fission products.

Out of that 0.6% only a small fraction are volatile species like Iodine-129 (I129).

Most is trapped in the ceramic pellet crystalline structure, with a small fraction available for release if the fuel were damaged during a transport accident.

Each fuel bundle is comprised of ceramic uranium fuel pellets, containing 19.2kg of Uranium, inside 37 zircaloy tubes that are welded shut (ie. half a kilo of uranium pellets in each tube).

After 50 years of storage, prior to shipment to a DGR, the amount of I129 in used fuel is 0.29 MBq/kgU (Where “MBq” stands for Mega-Becquerels or millions of Becquerels, and is listed per kilogram of Uranium (kgU) initially in the fuel bundles).

For comparison, the human body contains about 0.008 MBq of radioactivity, more than half of which is natural Potassium-40 (K40).

The United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR) use a dose conversion factor of 0.044 mSv/MBq for I129.

So, if ALL the I129 in a kilogram of used fuel were released and 100% of it absorbed by nearby people, the radiation dose they would receive (in milli-Sieverts, or “mSv”) would be 0.29 MBq/kgU x 0.044 mSv/MBq = 0.013 mSv (collective dose, not individual dose).

For comparison, the typical annual radiation dose Canadians get from natural background sources is between about 1.2 and 4 mSv, or roughly 150 times more (depending on where in Canada you live).

Of course in reality, only a tiny fraction of the I129 in that kilogram of used fuel could be released, and it’s extremely unlikely that anywhere near 100% of that would de absorbed by nearby people (or anything else).

Lastly, let’s remember that Iodine-129 occurs naturally in trace quantities in the environment, because uranium is ubiquitous in the ground and in oceans and lakes:

Somewhat like Radon gas, I129 comes from uranium, albeit in somewhat different ways.

While Radon is simply a decay product of uranium, I129 is produced by spontaneous fission of uranium, as well as fission due to neutrons in cosmic rays hitting uranium atoms.

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PS.  Readers here are invited to invited to join my “Rad Toolbox” group on Facebook: https://www.facebook.com/groups/150981218802374

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